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• W1984954832 abstract "Photoinduced charge separation and recombination to the triplet state in a carotene (C) porphyrin (P) fullerene (C 60 ) triad have been followed by time-resolved electron paramagnetic resonance (EPR). The electron transfer process has been studied at different temperatures in both a glassy isotropic matrix (2-methyltetrahydrofuran) and uniaxial liquid crystal (E-7). In both media, the triad undergoes two-step photoinduced electron transfer, with the generation of a long-lived charge separated state (C ” + -P-C 60 ” m ), and charge recombination to the triplet state, localized in the carotene moiety. The carotenoid triplet state is initially polarized according to the mechanism of recombination of a radical pair with singlet precursor. Both the photoinduced spin-correlated radical pair and the carotene triplet are observed in E-7 starting from the glass to the liquid crystal phase. The exchange interaction between the electrons in the radical pair (J=1.2 Gauss) has been evaluated by simulation of the EPR spectrum in the isotropic glass and comparison with the corresponding spectrum in the oriented medium." @default.
• W1984954832 created "2016-06-24" @default.
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• W1984954832 date "2003-01-01" @default.
• W1984954832 modified "2023-09-27" @default.
• W1984954832 title "Reaction Center Models in Liquid Crystals: Identification of Paramagnetic Intermediates" @default.
• W1984954832 cites W622652757 @default.
• W1984954832 doi "https://doi.org/10.1080/15421400390193648" @default.
• W1984954832 hasPublicationYear "2003" @default.
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