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- W1984966170 abstract "The replica Ornstein−Zernike equations, supplemented by the hypernetted chain approximation, were solved for size and/or charge asymmetric electrolytes adsorbed in a disordered matrix of charged species that are electroneutral in total. More precisely, the matrix was represented as a symmetric +1:−1 electrolyte. To obtain the numerical solution of the replica Ornstein−Zernike equations, renormalization of the initial equations was performed. Both the matrix and adsorbed fluid were modeled as charged hard spheres in a dielectric continuum. As a result of the numerical calculation, we obtained pair distribution functions. The effect of charge and size asymmetry of the annealed fluid was investigated. We present the results for charge asymmetric +2:−1 and +3:−1 electrolytes, and for a solution with asymmetries in charge of +3:−1 (+6:−1) and asymmetries in diameter of 7 Å:4 Å (20 Å:4 Å). In addition to the structural properties, the isothermal compressibility and the excess internal energy of the adsorbed electrolyte were calculated." @default.
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- W1984966170 date "1999-05-29" @default.
- W1984966170 modified "2023-09-26" @default.
- W1984966170 title "Structure and Thermodynamics of Asymmetric Electrolytes Adsorbed in Disordered Electroneutral Charged Matrices from Replica Ornstein−Zernike Equations" @default.
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- W1984966170 doi "https://doi.org/10.1021/jp990253i" @default.
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