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- W1985131985 abstract "In situ CW-EPR and diffuse reflectance UV−visible spectroscopy were used to monitor the spontaneous incorporation of ACENE-4 or tetracene (C18H12) in the medium-pore MnZSM-5 zeolites [Mn(AlO2)n(SiO2)96-n; MNa+, H+; n = 3.4, 6.6] by direct exposure under dry and inert atmosphere of solid ACENE-4 to dehydrated porous materials without any solvent. The sorption of the large ACENE-4 molecule with relatively low ionization potential (6.97 eV) occurs in Bronsted acidic HnZSM-5 zeolites according to a complex and slow reaction sequence including protonation, charge separation, hole transfer, and charge recombination while ACENE-4 is incorporated as an intact molecule in nonacidic NanZSM-5. After a long organization period, ACENE-4 lies in the straight channel in front of sodium cation in close proximity of Al framework atom as simulated by Monte Carlo calculations. The multivariate curve resolution (MCR) analysis of the huge DRUVv spectra set recorded during the ACENE-4 sorption course in acidic HnZSM-5 resolved..." @default.
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- W1985131985 date "2007-10-30" @default.
- W1985131985 modified "2023-09-26" @default.
- W1985131985 title "Spontaneous Charge Separation and Recombination Induced by Tetracene Incorporation in Pores of Acidic H<i><sub>n</sub></i>ZSM-5 Zeolites" @default.
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- W1985131985 doi "https://doi.org/10.1021/jp074607e" @default.
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