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- W1985280385 abstract "In this paper, treatment of N-(isonicotinoyl)-N‘-nicotinoylhydrazine (inh) and AgI with excess KI afforded a unique coordination polymeric cluster {[AgI(inh)]6(KI)}n (1) with the hexagram cluster units centered by μ6-I. In the polymer these hexagram units are parallel to the ab plane and are linked by separated K+ centers through inh. Polymer 1 represents the first example of coinstantaneous cation−anion-induced supramolecular self-assembly with nanoscale inner cavities. The polymer's third-order nonlinear optical (NLO) properties were determined by the Z-scan technique in DMF solution. The results show that the polymer has strong third-order optical nonlinearities. The nonlinear absorptive index a2 and refractive index n2 are calculated to be 1.044 × 10-9 mW-1 and 2.827 × 10-11 esu, respectively. The values are comparable to those of the reported cluster polymers. The optical limiting experiments show that the present cluster exhibits a large optical limiting capacity. The value of the limiting threshold was measured as 0.53 J cm-2 from the optical limiting experimental data. This value is three times better than 1.6 J cm-2 of C60. This paper also gives a summary and comparison on the optical limiting properties of oligomeric and polymeric clusters." @default.
- W1985280385 created "2016-06-24" @default.
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- W1985280385 date "2005-03-01" @default.
- W1985280385 modified "2023-09-30" @default.
- W1985280385 title "Synthesis, Structure, and Large Optical Limiting Effect of the First Coordination Polymeric Cluster Based on an {I@[AgI(inh)]<sub>6</sub>} Hexagram Block" @default.
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- W1985280385 doi "https://doi.org/10.1021/ic0487023" @default.
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