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• W1985622016 abstract "Results of quasielastic and inelastic incoherent neutron scattering experiments of light water at several thermodynamic states (200&lt;T&lt;400 °C and 184&lt;P&lt;400 bar) corresponding to densities ranging from 0.2 to 0.9 g/cm3 are presented. The results have been analyzed using a jump diffusion model and the two parameters of this model, namely, τ0, the residence time and D, the translational diffusion coefficient have been determined as a function of the density of supercritical water. The values of the diffusion coefficient D reported here are in very good agreement with those measured by NMR and increases strongly as the density of the medium decreases. The residence time τ0 slightly increases as the density of supercritical water decreases, with a value between 0.14 and 0.2 ps (ten times shorter than that measured in ambient liquid water). Moreover, we observe an almost linear increase in the mean jump distance L=6Dτ0 from 1.5 Å at 0.9 g/cm3 to 4 Å at 0.2 g/cm3. Finally, the value of the mean square displacement 〈u2〉1/2 increases from 0.6 Å at 0.9 g/cm3 to 1 Å at 0.2 g/cm3." @default.
• W1985622016 created "2016-06-24" @default.
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• W1985622016 date "2000-08-22" @default.
• W1985622016 modified "2023-09-25" @default.
• W1985622016 title "The dynamics of supercritical water: A quasielastic incoherent neutron scattering study" @default.
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• W1985622016 doi "https://doi.org/10.1063/1.1286599" @default.
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