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• W1985819786 abstract "An electron transfer reaction in a polar solvent has been considered in the region of the crossover from activation transfer to tunneling. An exact expression for the rate constant for an adiabatic potential surface has been found and has also been expressed in terms of a linear response theory for an arbitrary dielectric loss function of the solvent. The specific cases of electron transfer in water and inner-sphere electron transfer have been studied. The range for which quantum effects are important, in terms of the splitting between the adiabatic potential surfaces, has been found. The theory provides a simple numerical method for calculating the rate constant in this region using a few experimentally obtainable results. This is in contrast to previous methods where complex potential energy surfaces were required to numerically determine the rate." @default.
• W1985819786 created "2016-06-24" @default.
• W1985819786 creator A5054357219 @default.
• W1985819786 date "1993-11-15" @default.
• W1985819786 modified "2023-09-24" @default.
• W1985819786 title "Adiabatic electron transfer in polar solvents. Crossover from activation transfer to tunneling" @default.
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• W1985819786 doi "https://doi.org/10.1063/1.465701" @default.
• W1985819786 hasPublicationYear "1993" @default.
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