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- W1985878357 abstract "Hyper-Rayleigh scattering (HRS) of sulfosuccinate-based room-temperature ionic liquids (RTILs), tetraalkylammonium salts of bis(2-ethylhexyl)sulfosuccinate (BEHSS−) and di(isobutyl)sulfosuccinate (DIBSS−), shows strong orientation correlation between sulfosuccinate ions for both BEHSS−-based and DIBSS−-based RTILs. The hyperpolarizability and polarization resolved HRS, giving information at the dipolar electric order and at the quadrupolar electric order, respectively, have been measured as a function of the distance between sulfosuccinates by changing the size of the tetraalkylammonium ions constituting the ionic liquids. The variations obtained for the dipolar electric and quadrupolar electric components of the HRS intensity show the orientation correlation between sulfosuccinate ions. In particular, the weight parameter η introduced for molecular assemblies deviates from a pure dipolar electric order that is generally expected for a homogeneous molecular solution. Nonmonotonic variations of η with increasing the alkyl chain length of tetraalkylammonium ions indicate a transition in the organization of the anions from an homogeneous to an heterogeneous arrangement with increasing the intermolecular distance between sulfosuccinate ions due to the competition between the short- and long-range molecular interactions." @default.
- W1985878357 created "2016-06-24" @default.
- W1985878357 creator A5021257429 @default.
- W1985878357 creator A5023351527 @default.
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- W1985878357 date "2009-10-20" @default.
- W1985878357 modified "2023-10-18" @default.
- W1985878357 title "Orientation Correlation of Sulfosuccinate-based Room-Temperature Ionic Liquids Studied by Polarization-Resolved Hyper-Rayleigh Scattering" @default.
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- W1985878357 doi "https://doi.org/10.1021/jp907416m" @default.
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