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- W1985909627 abstract "Internuclear electronic interactions in conjugated ferrocene oligomers display unique redox and optical properties. I describe here recent research on the dependence of such properties on the number of ferrocene nuclei and on the structure of conjugated spacers. The neighboring-site interaction model explains the redox properties of oligo(ferrocene-1,1′-diyl)s. The infrared (IR) spectra of carbonyl complex-bound biferrocene and terferrocene enlighten the electronic structure in the mixed-valence states. Energy shifts of intervalence transfer (IT) in the mixed-valence states of oligo(ferrocene-1,1′-diyl)s resulting from changes in the oxidation state are rationalized by taking into account the change in neighboring-site combination by photo-electron transfer, which delivers extra energy due to the strain in internuclear distance. Oligo- and poly-(ferrocene-1,1′-diyl)s oxidized partially by tetracycanoethylene (TCNE) exhibit near-IR photoconductivity. Conjugated spacer groups between ferrocene nuclei involv..." @default.
- W1985909627 created "2016-06-24" @default.
- W1985909627 creator A5089786787 @default.
- W1985909627 date "2001-01-01" @default.
- W1985909627 modified "2023-10-17" @default.
- W1985909627 title "Redox and Optical Properties of Conjugated Ferrocene Oligomers" @default.
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- W1985909627 doi "https://doi.org/10.1246/bcsj.74.19" @default.
- W1985909627 hasPublicationYear "2001" @default.
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