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- W1986278431 abstract "Micro-Raman spectra of supersaturated aerosols of sodium succinate were obtained. The conformation behavior of the succinate dianion as a function of relative humidity (RH) was investigated by combining micro-Raman spectroscopy with theoretical calculations. A shoulder at 968 cm−1 of the v(C–CO2−) band on the rise in more concentrated droplets was believed indicative of conformation transformations. The intensity ratio (I963/I997) of the v(C–CO2−) band at 963 cm−1 to the v(C–C) band at 997 cm−1, versus the molar water-to-solute ratio (WSR), was used to fathom the equilibrium between gauche and trans conformations. Before saturation (WSR = 25.8) for the droplets, the ratio of I963/I997 retains a value of ∼2.6 independent of WSR, indicating that the equilibrium was not disturbed in the dilute droplets. In supersaturated droplets (WSR < 25.8), however, the ratio sharply decreases from ∼2.6 to ∼1.1 at WSR = 9.6, which was attributed to the formation of contact ion pairs (CIPs)." @default.
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- W1986278431 date "2008-01-01" @default.
- W1986278431 modified "2023-10-16" @default.
- W1986278431 title "Micro-Raman study on the conformation behavior of succinate in supersaturated sodium succinate aerosols" @default.
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- W1986278431 doi "https://doi.org/10.1039/b719457a" @default.
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