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• W1986943099 abstract "We have performed Monte Carlo simulations of homogeneous and heterogeneous nucleations of Lennard-Jones argon clusters. The simulation results were interpreted using the major concept posing a difference between the homogeneous and heterogeneous classical nucleation theories—the contact parameter. Our results show that the multiplication concept of the classical heterogeneous nucleation theory describes the cluster-substrate interaction surprisingly well even for small molecular clusters. However, in the case of argon nucleating on a rigid monolayer of fcc(111) substrate at T=60K, the argon-substrate atom interaction being approximately one-third as strong as the argon-argon interaction, the use of the classical theory concept results in an underestimation of the heterogeneous nucleation rate by two to three orders of magnitude even for large clusters. The main contribution to this discrepancy is induced by the failure of the classical theory of homogeneous nucleation to predict the energy involved in bringing one molecule from the vapor to the cluster for clusters containing less than approximately 15molecules." @default.
• W1986943099 created "2016-06-24" @default.
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• W1986943099 date "2006-10-26" @default.
• W1986943099 modified "2023-10-16" @default.
• W1986943099 title "Comparison between the classical theory predictions and molecular simulation results for heterogeneous nucleation of argon" @default.
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• W1986943099 doi "https://doi.org/10.1063/1.2358343" @default.
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