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• W1987143130 endingPage "4556" @default.
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• W1987143130 abstract "The optical absorption (OA) and photoluminescence (PL) spectra of pristine, oxygen-free ${mathrm{C}}_{60}$ films in the vicinity of the absorption edge across the highest-occupied-molecular-orbital to lowest-unoccupied-molecular-orbital (HOMO-LUMO) gap are studied to elucidate the nature of these electronic states. Structures observed in both the OA and PL spectra are identified with Herzberg-Teller vibronic coupling of the respective singlet electronic states to intramolecular vibrational modes. Similarities and differences among the PL and OA spectra of ${mathrm{C}}_{60}$ in solution, solid films, and single crystals are discussed. The larger linewidth of the ${mathrm{C}}_{60}$ film spectra is attributed to the presence of defects, presumably associated with numerous grain boundaries. Finally, the OA and PL spectra of photopolymerized ${mathrm{C}}_{60}$ solid films are presented. The features in both the OA and PL spectra are observed to broaden considerably. In addition, two of the OA bands blueshift slightly (400--800 ${mathrm{cm}}^{mathrm{ensuremath{-}}1}$) and the PL features downshift by ensuremath{sim}330 ${mathrm{cm}}^{mathrm{ensuremath{-}}1}$ upon polymerization. These results are consistent with the intermolecular oligomerization bond disorder and reduced symmetry of the ${mathrm{C}}_{60}$ shell imposed by the covalent bonds between ${mathrm{C}}_{60}$ molecules in the polymeric phase." @default.
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• W1987143130 date "1995-02-15" @default.
• W1987143130 modified "2023-10-16" @default.
• W1987143130 title "Optical absorption and photoluminescence in pristine and photopolymerized<mml:math xmlns:mml=http://www.w3.org/1998/Math/MathML display=inline><mml:mrow><mml:msub><mml:mrow><mml:mi mathvariant=normal>C</mml:mi></mml:mrow><mml:mrow><mml:mn>60</mml:mn></mml:mrow></mml:msub></mml:mrow></mml:math>solid films" @default.
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• W1987143130 doi "https://doi.org/10.1103/physrevb.51.4547" @default.
• W1987143130 hasPubMedId "https://pubmed.ncbi.nlm.nih.gov/9979301" @default.
• W1987143130 hasPublicationYear "1995" @default.
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