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• W1987457557 abstract "Until now, ultrafast IR spectroscopy has been limited by the bandwidth of optical parametric amplifiers, typically 100–400 cm−1. Here we present the first example of transient IR spectroscopy using a continuum laser source to probe the entire mid-IR region with ultrafast time resolution. The continuum source is based on focusing the fundamental, second harmonic, and third harmonic of 1 mJ, 25 fs, 800 nm pulses in air, generating ∼150 fs continuum mid-IR pulses that span the frequency range of <400 to >5000 cm-1 or, conversely, <2 to >25 μm. We characterize the spectral and temporal properties of dicarbonylacetonato rhodium(I) in hexane. We further demonstrate the versatility of the method by measuring the very fast and broad (>1500 cm-1) spectral changes following IR excitation associated with the 7-azaindole–acetic acid heterodimer in carbon tetrachloride." @default.
• W1987457557 created "2016-06-24" @default.
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• W1987457557 date "2012-06-06" @default.
• W1987457557 modified "2023-09-30" @default.
• W1987457557 title "Ultrafast continuum mid-infrared spectroscopy: probing the entire vibrational spectrum in a single laser shot with femtosecond time resolution" @default.
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• W1987457557 doi "https://doi.org/10.1364/ol.37.002265" @default.
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