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• W1987679902 abstract "Sub-picosecond pulses are used to measure the transient IR spectra of vibrationally excited Rh(CO) 2 (acac) in dilute solutions of n -hexane and CCl 3 H. Ground-state bleach and excited-state absorption features are observed at t D >0, while interference-like spectra characteristic of the perturbed free induction decay (FID) of the probe polarization are seen at t D <). At t D >), the bleach signal exhibits an initial decay ( n -hexane, 3–6 ps; CCl 3 H, 2.2–4 ps) attributed to rapid v-v coupling between the symmetric and asymmetric stretch modes of the dicarbonyl, followed by much slower ( n -hexane, 61 ps; CCl 3 H, 101 ps) population relaxation. Calculated transient spectra and bleach decay curves obtained from a 5-level density matrix model of the coupled CO oscillators account for the data, including the effects due to perturbed FID and rapid v-v coupling." @default.
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• W1987679902 date "1992-03-01" @default.
• W1987679902 modified "2023-09-25" @default.
• W1987679902 title "Sub-picosecond time-resolved IR spectroscopy of the vibrational dynamics of Rh (CO)2 (acac)" @default.
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• W1987679902 doi "https://doi.org/10.1016/0301-0104(92)80015-n" @default.
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