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- W1987699993 abstract "Given the convenient sealing of fiber-shaped dye-sensitized solar cells (FDSSCs), the electrolyte refreshing effect on the photo-electrochemical performance of FDSSCs was studied. The electron transport and interfacial recombination kinetics were also systematically investigated by electrochemical impedance spectroscopy. With increased electrolyte refreshing times from 0 to 10, the open-circuit voltage (<mml:math xmlns:mml=http://www.w3.org/1998/Math/MathML><mml:msub><mml:mrow><mml:mi>V</mml:mi></mml:mrow><mml:mrow><mml:mtext>o</mml:mtext><mml:mtext>c</mml:mtext></mml:mrow></mml:msub></mml:math>) and fill factor (FF) increased, whereas the photocurrent density (<mml:math xmlns:mml=http://www.w3.org/1998/Math/MathML><mml:msub><mml:mrow><mml:mi>J</mml:mi></mml:mrow><mml:mrow><mml:mtext>s</mml:mtext><mml:mtext>c</mml:mtext></mml:mrow></mml:msub></mml:math>) and power conversion efficiency (PCE) significantly decreased. The increased<mml:math xmlns:mml=http://www.w3.org/1998/Math/MathML><mml:msub><mml:mrow><mml:mi>V</mml:mi></mml:mrow><mml:mrow><mml:mtext>o</mml:mtext><mml:mtext>c</mml:mtext></mml:mrow></mml:msub></mml:math>was mainly ascribed to the electron recombination resistance (<mml:math xmlns:mml=http://www.w3.org/1998/Math/MathML><mml:msub><mml:mrow><mml:mi>R</mml:mi></mml:mrow><mml:mrow><mml:mtext>ct</mml:mtext><mml:mtext>, WE</mml:mtext></mml:mrow></mml:msub></mml:math>) at the TiO 2 /electrolyte interface and electron lifetime. The decreased<mml:math xmlns:mml=http://www.w3.org/1998/Math/MathML><mml:msub><mml:mrow><mml:mi>J</mml:mi></mml:mrow><mml:mrow><mml:mtext>s</mml:mtext><mml:mtext>c</mml:mtext></mml:mrow></mml:msub></mml:math>and PCE were due to dye desorption and the increase of series resistance. Further investigation proved that Li + played a vital role in increasing<mml:math xmlns:mml=http://www.w3.org/1998/Math/MathML><mml:msub><mml:mrow><mml:mi>V</mml:mi></mml:mrow><mml:mrow><mml:mtext>o</mml:mtext><mml:mtext>c</mml:mtext></mml:mrow></mml:msub></mml:math>as electrolyte refreshing and Li + had more significant impact than TBP (tert-butyl pyridine) on maintaining high<mml:math xmlns:mml=http://www.w3.org/1998/Math/MathML><mml:msub><mml:mrow><mml:mi>V</mml:mi></mml:mrow><mml:mrow><mml:mtext>o</mml:mtext><mml:mtext>c</mml:mtext></mml:mrow></mml:msub></mml:math>." @default.
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- W1987699993 date "2012-01-01" @default.
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- W1987699993 title "Influence of Electrolyte Refreshing on the Photoelectrochemical Performance of Fiber-Shaped Dye-Sensitized Solar Cells" @default.
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