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- W1987702110 abstract "Three aminoalkanethiols that have large electron-transfer rate constants, SH−(CH2)n−NH2 (n = 6, 8, and 11), were individually self-assembled on Au electrodes, followed by covalent attachment of tris(2,2′-bipyridyl)ruthenium(II) (Ru(bpy)32+) moieties onto the end of the thiols. Two separate electrogenerated chemiluminescence (ECL) waves were observed upon anodic potential scanning from 0 to 1.40 V vs Ag/AgCl (3 M KCl) over the electrode placed in 0.10 M tri-n-propylamine (TPrA)/0.10 M phosphate buffer (pH 7.4) solution. The first ECL wave, located at ∼0.88 V vs Ag/AgCl, was associated with the direct oxidation of TPrA at the electrode, and the second ECL wave, located at ∼1.12, 1.22, and 1.35 V vs Ag/AgCl for n = 6, 8, and 11, respectively, was directly related to the oxidation of the tethered Ru(bpy)32+ species. The electron transfer behavior through DNA was examined at Au electrodes, which were covalently immobilized with 15-mer and 20-mer single-stranded (ss) DNA, respectively, and then hybridized with ..." @default.
- W1987702110 created "2016-06-24" @default.
- W1987702110 creator A5055997770 @default.
- W1987702110 creator A5089592481 @default.
- W1987702110 date "2008-10-07" @default.
- W1987702110 modified "2023-09-27" @default.
- W1987702110 title "Examination of Electron Transfer Through DNA Using Electrogenerated Chemiluminescence" @default.
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- W1987702110 doi "https://doi.org/10.1021/jp805791p" @default.
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