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• W1988303343 endingPage "12233" @default.
• W1988303343 startingPage "12232" @default.
• W1988303343 abstract "Copper(I) and copper(II) 1,5-diaza-cis-decalin complexes [(N2)Cu] are effective precatalysts for aerobic oxidative coupling of naphthol substrates. Mechanistic studies, however, reveal that these complexes are not the reactive form of the catalyst under steady-state conditions. Rather, the active catalyst forms in a presteady-state self-processing step that involves oxygenation of the naphthol substrate. The oxygenated substrate, NapHOX, serves as a cofactor that combines with the (N2)Cu complexes to achieve highly selective, steady-state oxidase reactivity (aerobic oxidative biaryl coupling)." @default.
• W1988303343 created "2016-06-24" @default.
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• W1988303343 date "2008-08-19" @default.
• W1988303343 modified "2023-10-17" @default.
• W1988303343 title "Mechanistic Study of Asymmetric Oxidative Biaryl Coupling: Evidence for Self-Processing of the Copper Catalyst to Achieve Control of Oxidase vs Oxygenase Activity" @default.
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• W1988303343 doi "https://doi.org/10.1021/ja804570b" @default.
• W1988303343 hasPubMedCentralId "https://www.ncbi.nlm.nih.gov/pmc/articles/2897702" @default.
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• W1988303343 hasPublicationYear "2008" @default.
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