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- W1988433110 abstract "Bis zu drei Stereozentren werden hochselektiv in einer neuen C,O-Cyclodialkylierung dilithiierter 1,3-Dicarbonylverbindungen mit 1,4-Dibrom-2-buten aufgebaut. Diese Reaktion eröffnet einen effizienten regio- und stereoselektiven Zugang zu einer großen Bandbreite von 2-Alkyliden-5-vinyltetrahydrofuranen (ein Beispiel ist im Schema gezeigt). Diese konnten durch eine neuartige Pd-katalysierte Umlagerung in funktionalisierte Bicyclo[3.2.1]octan-8-one überführt werden, deren Grundgerüst in vielen pharmakologisch relevanten Naturstoffen vorkommt. LDA=Lithiumdiisopropylamid, dppe=1,2-Bis(diphenylphosphanyl)ethan, DMSO=Dimethylsulfoxid." @default.
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- W1988433110 date "2000-09-01" @default.
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- W1988433110 title "Stereoselektive Synthese und Pd-katalysierte Transformationen von 2-Alkyliden-5-vinyltetrahydrofuranen" @default.
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