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• W1989157079 abstract "A hydrodynamic theory has been developed for the diffusion and convection of linear, flexible macromolecules through cylindrical pores of molecular dimensions. A random coil macromolecule is modeled as a porous body, whose average shape and solvent permeability distribution are affected by confinement in a pore. To examine the effects of molecular configuration on hindered transport, the results were compared to those of a hydrodynamic theory for solid, spherical solutes. Although predicted hydrodynamic resistances to solute motion in pores tend to be lower for flexible macromolecules than for solid spheres, the less favorable partitioning of random coils between pores and bulk solution leads to lower transport rates for coils than spheres, for the same Stokes-Einstein radius and external driving force. This conclusion holds for both diffusion and convection, over a wide range of solute-to-pore size ratios. The effects of solvent quality and the polymer chain microstructure on the hindrance factors are considered, and the implications of recent data from hindered transport experiments discussed." @default.
• W1989157079 created "2016-06-24" @default.
• W1989157079 creator A5024256224 @default.
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• W1989157079 date "1988-01-01" @default.
• W1989157079 modified "2023-10-15" @default.
• W1989157079 title "Hydrodynamic theory for the hindered transport of flexible macromolecules in porous membranes" @default.
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• W1989157079 doi "https://doi.org/10.1016/s0376-7388(00)82442-4" @default.
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