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• W1990066689 abstract "While β-ketoesters are useful Michael donors, they were previously ineffective in Michael−Michael cascade reactions using α,β-unsaturated aldehydes in conjunction with diphenylprolinol silyl ether organocatalysts. However, through rational modification of substrates and manipulation of the catalytic cycle, we developed an efficient Michael−Michael cascade reaction using β-ketoesters of type 9. In this transformation, highly substituted fused carbocycles are generated in a single step in up to 87% yield and 99% ee." @default.
• W1990066689 created "2016-06-24" @default.
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• W1990066689 date "2009-11-18" @default.
• W1990066689 modified "2023-09-23" @default.
• W1990066689 title "A New Organocatalyzed Michael−Michael Cascade Reaction Generates Highly Substituted Fused Carbocycles" @default.
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• W1990066689 doi "https://doi.org/10.1021/ol9024293" @default.
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