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- W1990153037 abstract "We have synthesized two types of methoxyphenol thiols, Fc-MP1 and Fc-MP2 to use them in a voltammetric pH sensor. The methoxyphenol group was oxidatively triggered to o-quinone. Thus formed dyad molecules made possible pH measurements based on the pH-dependence of formal potential difference between quinone (pH indicator) and ferrocene (pH reference) moieties. Precise pH measurements over a wide pH range were possible even in a two-electrode mode without a reference electrode. The large polarization effect found in metal counter electrodes such as Au and Pt was removed by simply forming a mixed monolayer using an inert alkanethiol as a diluent. Fc-MP1 and Fc-MP2 were complementary in that Fc-MP2 covers the pH region that was not accessed by Fc-MP1 because of the potential overlap between the Fc+/Fc and Q/H2Q redox processes. The estimated errors were in the range of 0.03 to 0.06 pH units from the analysis of varience." @default.
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- W1990153037 date "2013-01-01" @default.
- W1990153037 modified "2023-10-02" @default.
- W1990153037 title "Triggerable single-component two-electrode voltammetric pH sensors using dyad molecules" @default.
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- W1990153037 doi "https://doi.org/10.1016/j.elecom.2012.10.025" @default.
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