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• W1990229508 abstract "We review recent work in the study of interfacial electronic states and electron–adsorbate interactions with time- and angle-resolved two-photon photoemission (2PPE) spectroscopy. Results for interfaces between noble-metal surfaces and organic as well as inorganic dielectric overlayers are presented. Layer structure and thickness have pronounced effects on the spatial extents, binding energies, and dynamics of image-potential states (IPS) and molecular orbitals. The transition from delocalized to localized states in the plane of the interface can also occur dynamically through electron-induced nuclear motion in the overlayer. An important example of this class of phenomenon is the formation of polaronic states from initially delocalized IPS, which occurs on sub-picosecond timescales. Dynamic energy relaxation through electron solvation by molecular dipoles, the analogue of the dynamic Stokes shift in bulk solvents, may also accompany localization on ultrafast timescales, and has become the focus of much recent experimental and theoretical interest. The interplay of a static layer structure and an evolving potential from the adsorbate creates a rich environment for interfacial electron dynamics, as evidenced by the alcohol/Ag(1 1 1), nitrile/Ag(1 1 1), and D2O/Cu(1 1 1) systems. We conclude with a discussion of recent attempts to determine the spatial extent of localization parallel to the interface for electrons following localization and solvation using experimental measurements of the photoelectron distribution in momentum space." @default.
• W1990229508 created "2016-06-24" @default.
• W1990229508 creator A5012832287 @default.
• W1990229508 creator A5031809484 @default.
• W1990229508 creator A5047386130 @default.
• W1990229508 date "2005-01-01" @default.
• W1990229508 modified "2023-09-27" @default.
• W1990229508 title "Time- and angle-resolved two-photon photoemission studies of electron localization and solvation at interfaces" @default.
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