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• W1990335783 abstract "The phosphatriafulvenes 3a,b , accessible from the cyclopropenone 1 and the lithium phosphides 2 , possess inverse electron density as indicated by structure B ; this can also be deduced from ab initio calculations. In accord with the electronic structure, methyllithium attacks at a carbon atom of the three-membered ring (to 4 5 ), carboxylic acid chlorides effect P -acylation (to 6 ), and dimethyl acetylenedicarboxylate inserts into the P/Si bond (to 8 ). Condensation of di-tert-butylcyclopropenone with lithium silylphosphides yields phosphatriafulvenes, the first all carbon substituted phosphaalkenes with inverse electron densities. Ab initio calculations, NMR data and chemical reactions are in harmony with the concept." @default.
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• W1990335783 date "1989-01-01" @default.
• W1990335783 modified "2023-10-16" @default.
• W1990335783 title "Phosphatriafulvenes - phosphaalkenes with inverse electron density" @default.
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• W1990335783 doi "https://doi.org/10.1016/s0040-4039(01)93461-6" @default.
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