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• W1990337908 abstract "General peculiarities in the formation of quasibound complexes (QC) in collisions of an atom with a rigid diatomic or linear polyatomic molecule are studied using the method of classical trajectories. The CO2–Ar system is taken as an example. Statistical distributions of parameters characterizing either the formation of QC or those appropriate to rotational relaxation cross-sections are simulated and analyzed. Various factors are examined as far as their role in the formation of the QC is concerned: (1) the complexity of a trajectory approach (exact classical, planar, coplanar); (2) the selection of intermolecular potential energy surface (ab initio Parker–Snow–Pack potential; empirical Berreby–Dayan potential); (3) the departure of the initial CO2 rotational distribution from equilibrium. The cross-sections and bimolecular thermal rates for QC formation are obtained using the modified Sorbie–Murrell model. The use of derived analytical expressions makes the computations of QC fractions in CO2–Ar collisions easier both in equilibrium and in rotational non-equilibrium conditions." @default.
• W1990337908 created "2016-06-24" @default.
• W1990337908 creator A5057755153 @default.
• W1990337908 date "2004-08-20" @default.
• W1990337908 modified "2023-10-16" @default.
• W1990337908 title "Peculiarities of atom–quasidiatom collision complex formation: classical trajectory study" @default.
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• W1990337908 doi "https://doi.org/10.1080/0026897042000274766" @default.
• W1990337908 hasPublicationYear "2004" @default.
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