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• W1990487910 abstract "Abstract The oxidation state and coordination number of immobilized iron catecholate EtO 2 Fe(CAT‐POP) were determined by X‐ray absorption spectroscopy (XAS) under a variety of conditions. We find the as‐prepared material to be three‐coordinate Fe 2+ that readily oxidizes to Fe 3+ upon exposure to air but remains three‐coordinate. Both the reduced and oxidized Fe(CAT‐POP) catalyze olefin hydrogenation in batch and flow reactors. We determined the catalytic rates for both species and also observed by means of XAS that the oxidation state of the iron centers does not change in hydrogen at the reaction temperature. Therefore, we postulate that the mechanism of hydrogenation by Fe(CAT‐POP) proceeds through one of several possible nonclassical mechanisms, which are discussed." @default.
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• W1990487910 date "2013-07-12" @default.
• W1990487910 modified "2023-10-18" @default.
• W1990487910 title "In Situ X‐ray Absorption Spectroscopy and Nonclassical Catalytic Hydrogenation with an Iron(II) Catecholate Immobilized on a Porous Organic Polymer" @default.
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• W1990487910 doi "https://doi.org/10.1002/ejic.201300528" @default.
• W1990487910 hasPublicationYear "2013" @default.
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