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Matches in SemOpenAlex for { <https://semopenalex.org/work/W1990508698> ?p ?o ?g. }

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• W1990508698 abstract "We present a quasielastic neutron scattering (QENS) study of single-particle dynamics in pure water, measured at temperatures between 256 and 293 K along an isobaric path at 200 MPa. A thorough analysis of the spectral line shapes reveals a departure from simple models of continuous or jump diffusion, with such an effect becoming stronger at lower temperatures. We show that such a diverging trend of dynamical quantities upon cooling closely resembles the divergent (anomalous) compressibility observed in water by small-angle diffraction. Such an analogy suggests an interesting interplay between single-particle diffusion and structural arrangements in liquid water, both bearing witness of the well-known water anomalies. In particular, a fit of dynamical parameters by a Vogel−Tammann−Fulcher law provides a critical temperature of about 220 K, interestingly close to the hypothesized position of the second critical point of water and to the so-called Widom line." @default.
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• W1990508698 date "2010-11-29" @default.
• W1990508698 modified "2023-10-17" @default.
• W1990508698 title "Interplay between Microscopic Diffusion and Local Structure of Liquid Water" @default.
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• W1990508698 doi "https://doi.org/10.1021/jp1073768" @default.
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