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W1990575310 abstract "The Au–Ar complex is reinvestigated employing resonance-enhanced multiphoton ionization spectroscopy. Spectra are reported, corresponding to the atomic transition Au(6p←6s). This electronic excitation yields Π2 and Σ+2 states of Au–Ar, which interact under the influence of spin-orbit coupling. The spectra are consistent with strong σ-π mixing induced by the large spin-orbit coupling of Au, leading to strong interaction of the two Ω=1∕2 states, which arise from the Ar(S01)+Au(P1∕2,3∕22) asymptotes, and the consequent formation of a “shelf” on the outer wall of the lowest Ω=1∕2 state. In addition, high-level ab initio calculations are reported on the ground electronic state, X̃Σ+2, including extrapolation to the basis set limit." @default.
W1990575310 created "2016-06-24" @default.
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W1990575310 date "2007-11-28" @default.
W1990575310 modified "2023-10-16" @default.
W1990575310 title "Reinvestigation of the electronic spectroscopy of the Au–Ar complex" @default.
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W1990575310 doi "https://doi.org/10.1063/1.2800006" @default.
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