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- W1990675025 abstract "During oxidation of a lead electrode in a solution at potentials between −200 and +900 mV (vs. electrode) an anodic layer containing and is formed. When oxidation is conducted in the dark, does not display photoelectrochemical properties. In order to constitute a photoelectrochemical system the electrode has to be photoactivated by illumination with a given quantity of light at potentials more positive than 0 mV. In this case the layer converts into a layer with . When a photoactivated electrode is illuminated three types of photoelectrochemical processes occur. The first type leads to photoionization of lead oxide and and are evolved at the interface. These processes take place at potentials between −400 and 0 mV. The second kind occurs at potentials more positive than 0 mV and leads to the formation of and photoactivation of the oxide. The mechanism according to which these processes take place includes the formation of Pb4+ ions in the oxide via photochemical reactions, reconstruction of the unit cell of into that of containing oxygen vacancies, and reactions of these vacancies with water with the subsequent formation of . The third kind of photoprocesses leads to photolysis of water at the surface of the layer with formation of ." @default.
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- W1990675025 date "1977-10-01" @default.
- W1990675025 modified "2023-10-12" @default.
- W1990675025 title "Photoelectrochemical Properties of the Lead Electrode during Anodic Oxidation in Sulfuric Acid Solution" @default.
- W1990675025 doi "https://doi.org/10.1149/1.2133105" @default.
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