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- W1990720376 abstract "We have ignited mixtures of hydrogen, oxygen, and ozone in closed cells with 248 nm radiation from a KrF excimer laser. Ozone, the only significant absorber in this system, absorbs a single photon and produces oxygen atoms which initiate combustion. A discretized, time-dependent Beer's law model is used to demonstrate that the radical concentration immediately after photolysis is a function of laser power, ozone concentration, focal length, and separation between the lens and reaction cell. Spark schlieren photographs are used to visualize the ignition events and identify the ignition sites. The effects of equivalence ratio, pressure, and the initial gas temperature on the minimum ozone concentration needed to produce ignition are presented, and only the initial temperature has a significant effect. Modeling studies of the ignition process aid in the interpretation of the experimental results, and show that the ignition we observe is not due solely to thermal effects, but is strongly dependent on the number and type of radicals present initially after photolysis. Ignition using other hydrocarbons as fuels was also demonstrated." @default.
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- W1990720376 date "1987-08-01" @default.
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- W1990720376 title "Ignition by excimer laser photolysis of ozone" @default.
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- W1990720376 doi "https://doi.org/10.1016/0010-2180(87)90029-0" @default.
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