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• W1990838724 abstract "Using single molecule spectroscopy, we show that the fluorescence lifetime trajectories of single probe molecules embedded in a glass-forming polymer melt exhibit strong fluctuations of a hopping character. Using molecular dynamics simulations targeted to explain these experimental observations, we show that the lifetime fluctuations correlate strongly with the average square displacement function of the matrix particles. The latter observable is a direct probe of the meta-basin transitions in the potential energy landscape of glass-forming liquids. We thus show here that single molecule experiments can provide detailed microscopic information on system properties that hitherto have been accessible via computer simulations only." @default.
• W1990838724 created "2016-06-24" @default.
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• W1990838724 date "2006-11-22" @default.
• W1990838724 modified "2023-10-03" @default.
• W1990838724 title "Fluorescence Lifetime of a Single Molecule as an Observable of Meta-Basin Dynamics in Fluids Near the Glass Transition" @default.
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• W1990838724 doi "https://doi.org/10.1103/physrevlett.97.217801" @default.
• W1990838724 hasPubMedId "https://pubmed.ncbi.nlm.nih.gov/17155773" @default.
• W1990838724 hasPublicationYear "2006" @default.
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