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- W1991002925 abstract "Supertetrahedral compounds of chalcogenometalates (T3 cluster compounds) integrated with Ni-bpy (bpy = 2,2′-bipyridine) complex were prepared by a solvothermal technique. The compound [Ni(bpy)3]3[H4In10S20]·bpy·2EG·6H2O (Mb-InS-1) (EG = ethylene glycol) consists of discrete T3 clusters of [H4In10S20]6− with three [Ni(bpy)3]2+ cations. The compound [Ni(bpy)3]2[H2In10S19]·bpy·2HEA·2H2O (Mb-InS-2) (EA = ethanolamine) is a 1-D polymer, in which zigzag T3 cluster chains are charge balanced by metal-bpy complex cations. The compound [Ni(bpy)3]7[H4In40S74]·7Hbpy·3HEA·8H2O (Mb-InS-3) is a 2-D T3 polymer with cation layers of [Ni(bpy)3]2+. Integrating M-bpy complex cations into chalcogenido structures has been made with the aim of improving the photoabsorption of the materials. The electronic spectra showed the new bands of cation–anion charge-transfer (CACT) that is mainly caused by the S⋯H–C(py) contacts between the InS T3 supertetrahedral clusters and the [Ni(bpy)3]2+ cations." @default.
- W1991002925 created "2016-06-24" @default.
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- W1991002925 date "2011-01-01" @default.
- W1991002925 modified "2023-09-25" @default.
- W1991002925 title "Indium sulfide clusters integrated with 2,2′-bipyridine complexes" @default.
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- W1991002925 doi "https://doi.org/10.1039/c1dt10153f" @default.
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