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- W1991115304 abstract "We present a review of our recent work concerning the spin state of Fe2+ and Fe3+ in iron magnesium aluminium silicate perovskite, the most abundant phase in the Earth's interior. Experimental results obtained using Mössbauer spectroscopy (with a radioactive source and a Synchrotron Mössbauer Source) and nuclear forward scattering for a range of different sample compositions in both externally heated and laser-heated diamond anvil cells show clear trends in the variation of hyperfine parameters with pressure and temperature. These trends combined with reported total spin state measurements using X-ray emission spectroscopy on samples of similar composition support the conclusion that Fe2+ undergoes a high-spin to intermediate-spin transition near the top of the lower mantle and an intermediate-spin to low-spin transition near the bottom of the lower mantle. No spin transition is observed to occur in Fe3+ for samples with compositions relevant for the lower mantle." @default.
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- W1991115304 date "2013-06-11" @default.
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- W1991115304 title "Iron spin state in silicate perovskite at conditions of the Earth's deep interior" @default.
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- W1991115304 doi "https://doi.org/10.1080/08957959.2013.805217" @default.
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