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- W1991331454 abstract "At the station Kollumerwaard (The Netherlands), for monitoring tracers in the troposphere, air is sampled in 16 containers for off-line 13 C, 18 O and 14 C isotopic analysis of CO 2 . The timing of the sampling is chosen such that CO 2 variations correlating with pollutants like CO and CH 4 are optimally covered. The 14 C measurements enable us to discriminate between biospheric and fossil fuel contributions to atmospheric CO 2 . The analysis of one series sampled on 23 November 1994 resolves the increased CO 2 mixing ratio into a purely biospheric component with a δ 13 C of (− 22.2 ± 1.5)‰, and a fossil component of up to 35 ppm with a δ 13 C of (− 34.1 ± 1.6)‰. Another series, recorded on 2 and 3 February 1995, shows a nearby emission of fossil CO 2 , methane and carbon monoxide, most likely due to the flaring of natural gas. Both events clearly indicate the importance of natural gas consumption in or in the vicinity of Holland. These experimental values can be compared with estimates of CO 2 emissions from combustion of fossil fuels and the corresponding δ 13 C values. The results for 18 O show the pronounced difference in behaviour between the O and C isotopes in atmospheric CO 2 , due to the fast isotopic exchange processes with (plant, soil or ocean) water. As a side result, the method produces the ratio CO: fossil CO 2 , a direct measure for combustion quality on a regional scale. DOI: 10.1034/j.1600-0889.1996.00013.x" @default.
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- W1991331454 date "1996-09-01" @default.
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- W1991331454 title "Isotopic characterisation of CO2 sources during regional pollution events using isotopic and radiocarbon analysis" @default.
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- W1991331454 doi "https://doi.org/10.1034/j.1600-0889.1996.00013.x" @default.
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