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• W1991397997 startingPage "3444" @default.
• W1991397997 abstract "We study polymer reaction kinetics at interfaces. The interface of width $h$ increments the effective dimensionality by 1: Rate constants $k$ obey scaling laws as for 4-dimensional bulk reaction problems. For groups with small reactivity $Q$, $kensuremath{sim}h$ and is independent of molecular weight $N$. For large $Q$, $kensuremath{sim}frac{1}{mathrm{ln}N}$ and $kensuremath{sim}frac{1}{Nmathrm{ln}N}$ for unentangled and entangled polymers, respectively, with weak $h$ dependence. Consistent with recent experiments, we find $k$ is exponentially suppressed when copolymer product attains surface densities above a critical level, ${ensuremath{rho}}_{s}^{mathrm{crit}}ensuremath{sim}frac{1}{{N}^{frac{1}{2}}}$." @default.
• W1991397997 created "2016-06-24" @default.
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• W1991397997 date "1996-04-29" @default.
• W1991397997 modified "2023-09-27" @default.
• W1991397997 title "Polymer Reaction Kinetics at Interfaces" @default.
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• W1991397997 doi "https://doi.org/10.1103/physrevlett.76.3444" @default.
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