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• W1991452898 abstract "The use of a new method of preparing micron‐thick deposits of nanocrystals of ice for Fourier transform infrared sampling, with the nanocrystals supported on a vertical infrared window, has greatly improved the signal‐to‐noise levels of the spectra available for large ice clusters. High quality spectra of modes of the surface molecules are reported, even for regions that underlie the intense bands of the bulk ice modes. These experimental features are most clearly displayed through the use of difference spectra. For example, the difference between spectra obtained for nanocrystals, before and after an annealing cycle that significantly increases the average cluster size, reflects the decrease in number of surface groups and the corresponding increase in number of interior molecules. Similarly, differences between spectra of bare and adsorbate‐covered nanocrystals, obtained at the same temperature for the same ice sample, show the significant shifts of ‘‘surface‐localized’’ ice modes caused by the adsorbat..." @default.
• W1991452898 created "2016-06-24" @default.
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• W1991452898 date "1995-06-01" @default.
• W1991452898 modified "2023-10-18" @default.
• W1991452898 title "Infrared spectra of ice surfaces and assignment of surface‐localized modes from simulated spectra of cubic ice" @default.
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• W1991452898 doi "https://doi.org/10.1063/1.468825" @default.
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