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• W1991469424 abstract "The deliberate tailoring of nanostructured metallic catalysts at the monolayer-level is an ongoing challenge and could lead to new electronic and catalytic properties, since surface-catalyzed reactions are extremely sensitive to the atomic-level details of the catalytic surface. In this article, we present a novel electrochemical strategy to nanoparticle-based catalyst design using the recently developed underpotential deposition (UPD) redox replacement technique. A single UPD Cu replacement with Pt2+ yielded a uniform Pt layer on colloid gold surfaces. The ultrathin (nominally monolayer-level) Pt coating of the novel nanostructured particles was confirmed by cyclic voltammetry and X-ray photoelectron spectra (XPS). The present results demonstrate that ultrathin Pt coating effects efficiently and behaves as the nanostructured monometallic Pt for electrocatalytic oxygen reduction, and also shows size-dependent, tunable electrocatalytic ability. The as-prepared ultrathin Pt-coated Au nanoparticle monolayer ..." @default.
• W1991469424 created "2016-06-24" @default.
• W1991469424 creator A5003395657 @default.
• W1991469424 creator A5035360447 @default.
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• W1991469424 date "2004-05-20" @default.
• W1991469424 modified "2023-09-30" @default.
• W1991469424 title "Electrochemical Design of Ultrathin Platinum-Coated Gold Nanoparticle Monolayer Films as a Novel Nanostructured Electrocatalyst for Oxygen Reduction" @default.
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• W1991469424 doi "https://doi.org/10.1021/jp0375517" @default.
• W1991469424 hasPublicationYear "2004" @default.
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