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• W1991476163 abstract "The microscopic situations of ions, especially anions, adsorbed at metal/water and air/water interfaces are comparatively examined with regard to changes of ionic hydration that must be involved in so-called specific adsorption where short-range electronic chemisorptive int eractions arise with the electrode-metal surface. Specific adsorption of non-hydrophobic ions takes place usually with significant charge-transfer related to the electrosorption valency. In order for such electronic effects to arise through metal/lone-pair electron interactions, it is necessary for accompanying changes of solvation energy and of related geometry of the inner-shell solvent coordination of the ions to take place so that lone-pair orbitals eg on anions, can have access to emergent surface orbitals of the metal electrode. Correspondingly, the ion solvation factor is demonstrated by consideration of ion adsorption at air-water interfaces where the ion/metal electronic interaction is absent. In relation to the solvation factors, individual hydrated-ion properties are plotted vs. ionic crystal radii and show that such properties are differently sensitive to radii of anions in comparison with those of cations." @default.
• W1991476163 created "2016-06-24" @default.
• W1991476163 creator A5089825488 @default.
• W1991476163 date "1995-07-01" @default.
• W1991476163 modified "2023-10-14" @default.
• W1991476163 title "The solvation factor in specificity of ion adsorption at electrodes" @default.
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• W1991476163 doi "https://doi.org/10.1016/0013-4686(95)00031-9" @default.
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