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- W1991500982 abstract "Effect of reaction conditions on activity and product distribution on oxygenates formation during Fischer-Tropsch synthesis over a co-precipitated Fe-Cu-K-La/SiO2 catalyst was investigated. It showed that alcohols were the main components in total oxygenates. Selectivity of oxygenates decreased with temperature and increased with pressure. Reaction rate and overall oxygenates formation rate generally increased with temperature and pressure. It was found that oxygenates distribution was deeply dependent on reaction conditions. In-situ diffuse reflection infrared Fourier transform spectroscopy results showed that alkyl as well as methoxy species, which were thought to be a C1 product precursor, were greatly favored at high temperatures. An enhancement in alcohols and suppression in CO2 and CH4 with increasing pressure were also observed. Moreover, it was found that carbene was not the rate-controlling step in oxygenates synthesis." @default.
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- W1991500982 date "2014-07-24" @default.
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- W1991500982 title "Links between Reaction Intermediates, Reactivity, and Reaction Conditions in Oxygenates Formation during Fischer-Tropsch Synthesis" @default.
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- W1991500982 doi "https://doi.org/10.1080/15567036.2013.767864" @default.
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