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• W1991778046 abstract "As an extension to previous studies the methyl radical recombination reaction, CH3+CH3(+M)→C2H6(+M) (1) was studied behind reflected shock waves over the temperature range 1200–1600 K at total pressures of 10 to 240 bar with a 216.5 nm UV absorption spectroscopic technique. The reaction was in the falloff region under the conditions employed and the experimentally determined extinction coefficients of CH3 were found to be slightly pressure dependent at a fixed temperature. The extrapolated high-pressure limit rate constants could be well represented by (in cm3/mol s), k1∞=1.15×1015T−0.6, or k1∞=1.45×1013exp(330 K/T), or k1∞=5.36×1016T−1.1exp(−320K/T). A negative temperature dependence of k1∞ was therefore confirmed." @default.
• W1991778046 created "2016-06-24" @default.
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• W1991778046 date "1991-01-01" @default.
• W1991778046 modified "2023-10-01" @default.
• W1991778046 title "Recombination of CH3 radicals at elevated pressures and temperatures" @default.
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• W1991778046 doi "https://doi.org/10.1016/s0082-0784(06)80247-x" @default.
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