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- W1991966141 abstract "Abstract In this paper, we discuss the effects of the defect interactions on the thermodynamic properties and electronic transport of nonstoichiometric oxides. We first show that two limited thermodynamic behaviours can be distinguished depending on whether the oxide has a metallic type electronic conduction or a hopping electronic conduction. In the first case, the interactions are expected to be short ranged because of the screening of the conduction electrons, while they are Coulombic in the second case. This paper is limited to this last case, exemplified mainly by M1−xO(M=Co, Mn,…) cubic oxides. Next, we analyse the two approximated methods usally used in this field, the ideal mass action law method and the Debye Hückel theory, and we show that they are both insufficient to accurately describe these compounds. We finally show by means of Monte Carlo simulations that a simple model in which point defects interact through a unique dielectric constant allows us to render an account of the main features of the thermodynamic and electronic transport properties of these oxides." @default.
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- W1991966141 date "1995-12-01" @default.
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- W1991966141 title "Defect interactions, statistical thermodynamic and electronic transport in ionic nonstoichiometric oxides" @default.
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- W1991966141 doi "https://doi.org/10.1080/10420159508222728" @default.
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