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• W1992069728 abstract "A new thiolate/disulfide mediator was designed and synthesized by employing DFT calculations as a guide. It possesses high transparency to visible light, a very attractive feature for bifacially active transparent DSCs that require a highly transparent counter electrode (CE). Compared to the reported and most promising thiolate/disulfide mediator T−/T2, this new analogous mediator produced a major enhancement in open circuit potential (VOC) by about 40 mV and correspondingly a higher power conversion efficiency (η) for DSCs. Furthermore, a highly uniform and transparent (transmittance > 91%) poly(3,4-ethylenedioxythiophene) (PEDOTBE) CE was prepared and could efficiently catalyze the reduction of the disulfide. Based on the novel transparent redox couple and PEDOTBE CE, a new type of iodine-free and Pt-free transparent bifacial DSC was successfully fabricated. This new bifacial device could not only yield a promising front-illuminated η of 6.07%, but also produce an attractive η as high as 4.35% for rear-side irradiation, which exceeds the rear-illuminated η of 3.93% achieved for the same type of device, employing the dark-colored I−/I3− electrolyte." @default.
• W1992069728 created "2016-06-24" @default.
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• W1992069728 date "2012-01-01" @default.
• W1992069728 modified "2023-09-23" @default.
• W1992069728 title "Design of an organic redox mediator and optimization of an organic counter electrode for efficient transparent bifacial dye-sensitized solar cells" @default.
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• W1992069728 doi "https://doi.org/10.1039/c2cp43078a" @default.
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