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• W1992603272 abstract "Using nanosecond laser photolysis with 308 nm and Fourier transform EPR spectroscopy, the pyrimidine radicals (thymine, uracil and 6-methyluracil) generated by electron transfer from the pyrimidine ground state to spin-polarized anthraquinone-2,6-disulfonate (2,6-AQDS) triplets were studied. The pyrimidine radical cations decay by deprotonation at the N(1) position to the neutral pyrimidine-1-yl radical. No other reaction channel could be found. The rate constant of the electron transfer could be estimated from the triplet spin-polarization (CIDEP) of the 2,6-AQDS radical anions to: ket(thymine) = 4.1 × 109 M−1 s−1, ket(uracil) = 2.4 × 109 M−1 s−1 and ket(6-methyluracil) = 4.5 × 109 M−1 s−1." @default.
• W1992603272 created "2016-06-24" @default.
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• W1992603272 date "1997-09-01" @default.
• W1992603272 modified "2023-10-10" @default.
• W1992603272 title "Fourier transform EPR study of N-centered pyrimidine radicals in the nanosecond time-scale" @default.
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• W1992603272 doi "https://doi.org/10.1016/s0009-2614(97)00824-5" @default.
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