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• W1992612240 abstract "In this second paper of a two part series, we investigate the implications of the interfacial phenomenon, caused by adsorbate-adsorbate interactions coupled with the difference in adsorbate density between the zeolite and the gas phase, upon benzene permeation through single-crystal and polycrystalline microporous NaX membranes. The high flux predicted for thin single-crystal membranes reveals that substantially enhanced flux should be expected in submicron films. Simulations also indicate that the standard local equilibrium assumption made for larger scale membranes is inapplicable at the submicron scale associated with nanometer size grains of thin and/or polycrystalline membranes. Apparent activation energies predicted for benzene permeation through NaX membranes via kinetic Monte Carlo (KMC) simulations are in good agreement with laboratory experiments. The simulations also uncover temperature-dependent flux pathways leading to non-Arrhenius behavior observed experimentally. The failure of the Darken approximation, especially in the presence of the interfacial phenomenon, leads to a substantial overprediction of the flux. Simulations of polycrystalline membranes suggest that this same interfacial phenomenon leads to resistance that can reduce flux by an order of a magnitude with only moderate polycrystallinity." @default.
• W1992612240 created "2016-06-24" @default.
• W1992612240 creator A5003648678 @default.
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• W1992612240 date "2005-11-08" @default.
• W1992612240 modified "2023-09-27" @default.
• W1992612240 title "The role of molecular interactions and interfaces in diffusion: Permeation through single-crystal and polycrystalline microporous membranes" @default.
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• W1992612240 doi "https://doi.org/10.1063/1.2107415" @default.
• W1992612240 hasPubMedId "https://pubmed.ncbi.nlm.nih.gov/16292922" @default.
• W1992612240 hasPublicationYear "2005" @default.
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