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• W1992703519 endingPage "14363" @default.
• W1992703519 startingPage "14358" @default.
• W1992703519 abstract "The scattering of ${mathrm{H}}^{+}$ and ${mathrm{D}}^{+}$ ions from solid surfaces has been studied in a low-kinetic-energy region (50--500 eV), where the difference between these two projectiles can essentially be ascribed to their mass or velocity. It will be demonstrated that neutralization and inelastic scattering of ${mathrm{D}}^{+}$ are closely related to the bonding nature or the microscopic charge distribution of the solid surfaces. The neutralization of ${mathrm{D}}^{+}$ due to surface scattering from the ionic crystal (${mathrm{Sb}}_{2}$${mathrm{O}}_{3}$) is found to be small relative to that from the metal [Ta(111)] or the covalent materials [Si(111), ${mathrm{SiO}}_{2}$], indicating that the D 1s hole can readily diffuse into the ligands or the solid via the metallic or covalent orbital hybridizations while the isolated closed shell of the ionic crystal is not effective for hole diffusion. In ${mathrm{D}}^{+}$ scattering from the oxidized Ta(111) surface, the hole diffusion via the ionic O-Ta bond is suppressed while the metallic Ta-Ta bond retains high hole-diffusion efficiency. It is also concluded that oxygen chemisorption enhances reionization of neutral ${mathrm{D}}^{0}$ scattered after significant penetration into the solid, which contributes to the background in the ${mathrm{D}}^{+}$ energy spectra." @default.
• W1992703519 created "2016-06-24" @default.
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• W1992703519 date "1992-06-15" @default.
• W1992703519 modified "2023-10-06" @default.
• W1992703519 title "Chemical effects in low-energyD+scattering from oxides" @default.
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• W1992703519 doi "https://doi.org/10.1103/physrevb.45.14358" @default.
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