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- W1992785364 abstract "A quantum lattice dynamics treatment is presented for the angular degrees of freedom in molecular solids. Variational wavefunctions are chosen to span the whole range from high to low rotational barriers. The theory is applied to quadrupole forces in solid hydrogen, nitrogen and carbon dioxide. It is concluded that quadrupole forces provide a better description of anisotropic forces in nitrogen than in CO2. In the limit, the treatment gives a valid description of the librons in solid ortho-hydrogen." @default.
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- W1992785364 date "1972-03-01" @default.
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- W1992785364 title "Quantum mechanical treatment of librations (and librons) in molecular solids" @default.
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- W1992785364 doi "https://doi.org/10.1016/0009-2614(72)80097-6" @default.
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