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- W1992891038 abstract "Abstract Plutonium sesquicarbide was synthesized by the carbothermic reduction of dioxide both in vacuum and in flowing helium in order to investigate the mechanism and kinetics of its formation. The CO gas concentration during reduction in flowing helium was used to determine the rate of formation of sesquicarbide. For powder samples the reduction was found to be controlled by a surface reaction. For compacted samples the reduction was controlled by the diffusion of CO gas through the carbide layer. The activation energy was 375 and 385 kJ/mol for powder and compacted samples, respectively. It was inferred that three kinds of plutonium oxide, fcc PuO2 − x bcc Pu2O3, and hexagonal Pu2O3 exist as intermediate phases at 1680 K." @default.
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- W1992891038 date "1981-10-01" @default.
- W1992891038 modified "2023-09-26" @default.
- W1992891038 title "Synthesis of plutonium sesquicarbide by the reduction of dioxide with graphite" @default.
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- W1992891038 doi "https://doi.org/10.1016/0022-3115(81)90458-x" @default.
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