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- W1993055837 abstract "Combining double monochromator, tandem Fabry-Pérot interferometry (TFPI), and photon correlation spectroscopy (PCS), the full range of the dynamic susceptibility of the glass former o-terphenyl is covered (240–440 K). A time resolution of 6 ns is reached by the PCS setup, and the measuring gap between PCS and TFPI has significantly shrunk. Combined time domain data are presented, which cover 0.01 ps–100 s. Regarding the primary α-process, no recognizable change in shape and amplitude is observed, i.e., frequency-temperature superposition holds over the entire temperature range investigated. The only change in the susceptibility is the emergence of the excess wing contribution, leading to a flattening of the susceptibility minimum close to Tg. Separating relaxation contribution from fast and slow dynamics, we determine the relaxation strength 1−frel(T) of the fast dynamics, which shows a cusplike temperature dependence with a crossover temperature Tc=316±10 K. Due to relative small changes of 1−frel(T) the effect is difficult to identify in frel(T) itself. The crossover temperature is larger than previously reported as no extrapolation scheme is applied." @default.
- W1993055837 created "2016-06-24" @default.
- W1993055837 creator A5084946358 @default.
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- W1993055837 date "2010-09-28" @default.
- W1993055837 modified "2023-09-25" @default.
- W1993055837 title "Light scattering study on the glass former o-terphenyl" @default.
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- W1993055837 doi "https://doi.org/10.1063/1.3478533" @default.
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