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• W1993079200 abstract "Pure rotational transitions of a rare gas atom–reactive open-shell triatom van der Waals complex Ar–HO2 have been observed by Fourier transform microwave spectroscopy. The transitions observed are of a type with Ka=0 and 1. Furthermore, by monitoring the change of the free induction decay signal of the a-type transitions, b-type transitions have been observed by a double resonance technique in the region 18–49 GHz. All these transitions provide us precise molecular constants. The r0 structure of Ar–HO2 has been determined by fixing the structure of the HO2 monomer. The determined structure is planar and almost T shaped, where the argon atom is slightly shifted to the hydrogen atom of HO2. The experimental data supplemented by high-level ab initio calculations indicate that the van der Waals bond of Ar–HO2 is relatively rigid. On the other hand, effects on the unpaired electron distribution by the complex formation are found to be fairly small, since the fine and hyperfine constants of Ar–HO2 are well explained by those of the HO2 monomer." @default.
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• W1993079200 date "2005-05-06" @default.
• W1993079200 modified "2023-10-03" @default.
• W1993079200 title "Microwave and millimeter-wave spectroscopy of the open-shell van der Waals complex Ar–HO2" @default.
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• W1993079200 doi "https://doi.org/10.1063/1.1889429" @default.
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