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- W1993200426 abstract "Relative stabilities (ΔGc) of ammonium-bound monomers and dimers of anomeric β-d-pentofuranosyl 1α- and 1β-azide derivates are determinate using the kinetic method by measuring relative rates of competitive collision-induced dissociations of dimeric [ANH4B]+ and trimeric [A2NH4B]+ or [ANH4B2]+ cluster ions. Comparison between calculated ammonium affinities (AAs) and relative stabilities (ΔGc) of ammonium-bound monomers shows qualitative correlations between both thermochemical quantities, but in two examples the activation barrier differences of competitive fragmentation channels cause a large disparity between both thermochemical data. Therefore, the most stable ammonium-bound monomers of the anomeric lα- and lβ-2,3,5-tri-O-benzyl-β-d-arabino-pento-furanosyl azides possess the lowest ammonium affinities and the highest relative stabilities. Two different relative stabilities measured for the same ammonium-bound homo- or hetero-dimers indicate dissimilar activated barriers of trimers transition states for dimer formations. The activated barriers of trimers depend on the relative stabilities of ammonium-bound monomer within the trimeric cluster ions." @default.
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- W1993200426 date "2003-12-01" @default.
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- W1993200426 title "Characterization of anomeric differences of ammonium-bound monomeric and dimeric complex ions of 1α- and 1β-azido-pentofuranosyl derivates by kinetic method" @default.
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- W1993200426 doi "https://doi.org/10.1016/j.ijms.2003.08.014" @default.
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