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- W1993317480 abstract "The strongly restricted orientational motion of CO molecules trapped in the Xe4 internal cavity of myoglobin mutant L29W-S108L is investigated by polarization-dependent mid-infrared pump-probe spectroscopy at cryogenic temperatures. Following an ultrafast initial decay, the signal anisotropy reaches an asymptotic value that is significantly larger than the prediction from the well-known relation r=25⟨P2[μ⃗(0)∙μ⃗(τ)]⟩, based on previously established potential parameters. This discrepancy is explained by showing that the full four-point correlation function describing third-order spectroscopy ⟨μ⃗(0)μ⃗(0)μ⃗(τ)μ⃗(τ+t)⟩ does not factorize in systems where its fast decay is dominated by restricted reorientation of the transition dipole moments." @default.
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- W1993317480 date "2005-03-22" @default.
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- W1993317480 title "Restricted rotational motion of CO in a protein internal cavity: Evidence for nonseparating correlation functions from IR pump-probe spectroscopy" @default.
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- W1993317480 doi "https://doi.org/10.1063/1.1867352" @default.
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