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- W1993403952 abstract "A method is presented for determining the population A(0)0, the quadrupole alignment factors A(2)0, A(2)1, A(2)2, and the hexadecapole alignment factors A(4)0, A(4)1, A(4)2, A(4)3, A(4)4 for a (v,J) ground state distribution of a diatomic molecule probed by linearly polarized two-photon nonresonant excitation. General expressions are developed for the O, P, Q, R, and S branch transitions as a function of the rotational quantum number J. This treatment assumes that the resonant state reached by the two-photon transition is subsequently detected independent of its alignment. This can be achieved by 2+n multiphoton ionization in which the ionization steps are saturated, or by 2+1 laser induced fluorescence in which the fluorescence is collected independent of its polarization and spatial anisotropy. To extract the population and the eight alignment parameters the line intensities must be measured for several polarization settings of the laser beam. However, when the ground state distribution has cylindrical symmetry, only two alignment parameters are nonvanishing, A(2)0 and A(4)0, and they can be determined at a single polarization setting by comparing the line intensities of the different branches." @default.
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- W1993403952 date "1986-12-15" @default.
- W1993403952 modified "2023-10-14" @default.
- W1993403952 title "Determination of population and alignment of the ground state using two-photon nonresonant excitation" @default.
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- W1993403952 doi "https://doi.org/10.1063/1.451374" @default.
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